Requirements and Concepts for Waste Containers for Heat-Generating Radioactive Waste and Spent Fuel in Rock Salt, Claystone, and Crystalline Rock

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Requirements and Concepts for Waste Containers for Heat-Generating Radioactive Waste and Spent Fuel in Rock Salt, Claystone, and Crystalline Rock
Requirements and Concepts for Waste Containers for
Heat-Generating Radioactive Waste and Spent Fuel in

                                                                                                    ©2021 BGE TECHNOLOGY GmbH
Rock Salt, Claystone, and Crystalline Rock

Wilhelm Bollingerfehr, Ansgar Wunderlich (BGE TECHNOLOGY GmbH)
Sabine Prignitz (BGE Bundesgesellschaft für Endlagerung mbH)
Holger Völzke, Christian Herold, Dietmar Wolff (Bundesanstalt für Materialforschung und –prüfung)

                                  WMSymposia2021 | Wilhelm Bollingerfehr et. al.
Requirements and Concepts for Waste Containers for Heat-Generating Radioactive Waste and Spent Fuel in Rock Salt, Claystone, and Crystalline Rock
Context
 German Site Selection Act (StandAG) as of summer 2017:

  Repository systems for 3 host rock formations to be considered

                                                                                              ©2021 BGE TECHNOLOGY GmbH
        Rock salt, claystone and crystalline rock

  Type and total amount of expected heat generating waste:
        Waste from reprocessing:      approx. 8000 coquilles
        Spent nuclear fuel:           approx. 10,500 t of HM

  Waste container considered as a pivotal barrier of the entire repository system

 Question:
 How to correctly derive requirements for waste containers designed for HLW and SF?

March 11, 2021                            WMSymposia2021|Wilhelm Bollingerfehr, et. al.   1
Requirements and Concepts for Waste Containers for Heat-Generating Radioactive Waste and Spent Fuel in Rock Salt, Claystone, and Crystalline Rock
Status of HLW-Waste Container Development

                                                                                               ©2021 BGE TECHNOLOGY GmbH
 POLLUX® 10                                          POLLUX® 3
  real existing waste container                      idea of a waste container without any
   (prototype),                                        detailed planning
  manufactured on the basis of                       adjusted for a repository concept in
   detailed design calculations                        claystone

March 11, 2021                 WMSymposia2021|Wilhelm Bollingerfehr, et. al.              2
Requirements and Concepts for Waste Containers for Heat-Generating Radioactive Waste and Spent Fuel in Rock Salt, Claystone, and Crystalline Rock
Status of HLW-Waste Container Development

                                                                                               ©2021 BGE TECHNOLOGY GmbH
 POLLUX® 10                                          POLLUX® 3
  real existing waste container                      idea of a waste container without any
   (prototype),                                        detailed planning
  manufactured on the basis of                       adjusted for a repository concept in
   detailed design calculations                        claystone

March 11, 2021                 WMSymposia2021|Wilhelm Bollingerfehr, et. al.              3
Requirements and Concepts for Waste Containers for Heat-Generating Radioactive Waste and Spent Fuel in Rock Salt, Claystone, and Crystalline Rock
R&D-Project KoBrA
  In summer 2017 BMWi launched the R&D-Project:
  „Requirements and concepts for waste containers for the disposal of heat generating
  radioactive waste and spent nuclear fuel in rock salt, claystone and crystalline rock“

                                                                                           ©2021 BGE TECHNOLOGY GmbH
  („Anforderungen und Konzepte für Behälter zur Endlagerung von Wärme
  entwickelnden radioaktiven Abfällen und ausgedienten Brennelementen in Steinsalz,
  Tonstein und Kristallingestein“ – Acronym: KoBrA)

  Project partners:

   BAM (Bundesanstalt für Materialforschung und –prüfung), Berlin and
   BGE TECHNOLOGY GmbH, Peine (coordinator)

  Project duration: July 2017 to April 2020

March 11, 2021                    WMSymposia2021|Wilhelm Bollingerfehr, et. al.       4
Requirements and Concepts for Waste Containers for Heat-Generating Radioactive Waste and Spent Fuel in Rock Salt, Claystone, and Crystalline Rock
Work Program
  1. Survey of international existing requirements and concepts for waste container

                                                                                          ©2021 BGE TECHNOLOGY GmbH
  2. Identification of waste container-relevant boundary conditions and load parameter

  3. Derivation and compilation of requirements for waste containers

  4. Development of ideas and concepts for waste container designs

March 11, 2021                   WMSymposia2021|Wilhelm Bollingerfehr, et. al.        5
Requirements and Concepts for Waste Containers for Heat-Generating Radioactive Waste and Spent Fuel in Rock Salt, Claystone, and Crystalline Rock
Waste Container Worldwide
             Host rock               Container concept (Developers)                                    Description                             Status of development
                                                                                                                                               well advanced in the licensing
                            KBS-3                                                unshielded double-hull cask (cast-iron cask with solid        procedure (tests for production,
                            (SKB/Posiva Oy, Sweden, Finland)                     copper cladding) for fuel assemblies                          loading, sealing, transport,

                                                                                                                                                                                       ©2021 BGE TECHNOLOGY GmbH
                                                                                                                                               storage)
                                                                                                                                               concept study derived from KBS-
         Crystalline Rock   UOS                                                  unshielded double-hull cask made of different steels for fuel
                                                                                                                                               3
                            (Škoda, Czech Rep.)                                  assemblies
                                                                                                                                               ("KBS-3 made of steel")
                            UFC II                                               unshielded steel container with thin copper coating for      advanced concept (material,
                            (NWMO, Canada)                                       (CANDU) fuel assemblies                                      production and container tests)

                            Category C Container                                                                                              advanced concept (material,
                                                                                 unshielded steel canisters or fuel assemblies
                            (Andra, France)                                                                                                   production and container tests)
                            Supercontainer                                       steel cask for fuel assemblies or HLW canisters enclosed in
             Claystone                                                                                                                       Material tests
                            (ONDRAF/NIRAS, Belgium)                              concrete
                                                                                                                                              generic design for fuel
                                                                                                                                              assemblies and canisters
                            Reference container                                  unshielded, robust steel container for fuel assemblies or
                                                                                                                                              considered by RWM as a
                            (Nagra, Switzerland)                                 HLW canisters
                                                                                                                                              possible reference concept for
                                                                                                                                              final disposal containers in salt

                            BSK-3                                                                                                             Concept developed in R&D
                                                                                 unshielded steel canisters for the borehole storage of drawn
             Rock salt                                                                                                                        reports; emplace-ment
                            (GNS, Germany)                                       fuel rods or HLW canisters
                                                                                                                                              technology tested on dummy

                            POLLUX®-10                                                                                                          advanced concept (POLLUX®-8
                                                                                 shielded double-hull cask (steel and cast iron) for drawn fuel
                                                                                                                                                manufactured as prototype;
                            (GNS, Germany)                                       rods or HLW canisters
                                                                                                                                                storage technology tested)

                                                                                                                                              Existing containers;
                            Transport and Storage Casks, e.g. CASTOR®            shielded transport and interim storage casks made of cast
                 --                                                                                                                           suitability for final disposal not yet
                            (GNS, Germany)                                       iron or forged steel for fuel assemblies or HLW canisters
                                                                                                                                              considered

March 11, 2021                                            WMSymposia2021|Wilhelm Bollingerfehr, et. al.                                                                           6
Requirements and Concepts for Waste Containers for Heat-Generating Radioactive Waste and Spent Fuel in Rock Salt, Claystone, and Crystalline Rock
Waste Container Boundary Conditions
                                                                     2. concepts for a repository in claystone

                                                                                                                   ©2021 BGE TECHNOLOGY GmbH
1. concept for a repository in rocksalt

                                                                 German                       French
                                                                 Repository Concept           Repository Concept
                                                                 (R&D-Project: AnSicht)       (Source: Andra)
                            Source: SKB

         3. concept for a repository in
                crystalline rock
March 11, 2021                            WMSymposia2021|Wilhelm Bollingerfehr, et. al.                     7
Requirements and Concepts for Waste Containers for Heat-Generating Radioactive Waste and Spent Fuel in Rock Salt, Claystone, and Crystalline Rock
Waste Container Boundary Conditions
                                                                     2. concepts for a repository in claystone

                                                                                                                   ©2021 BGE TECHNOLOGY GmbH
1. concept for a repository in rocksalt
              But how to derive correctly a comprehensive set of requirements
                         for waste containers for different host rocks?

                                                                 German                       French
                                                                 Repository Concept           Repository Concept
                                                                 (R&D-Project: AnSicht)       (Source: Andra)
                            Source: SKB

         3. concept for a repository in
                crystalline rock
March 11, 2021                            WMSymposia2021|Wilhelm Bollingerfehr, et. al.                     8
Requirements and Concepts for Waste Containers for Heat-Generating Radioactive Waste and Spent Fuel in Rock Salt, Claystone, and Crystalline Rock
Methodological Approach

                                                                        ©2021 BGE TECHNOLOGY GmbH
March 11, 2021      WMSymposia2021|Wilhelm Bollingerfehr, et. al.   9
Methodological Approach

                                                                                             ©2021 BGE TECHNOLOGY GmbH
                                           The idea is to:
                 •   Start with a compilation of requirements (regulatory, etc.)
                 •   Consider the lifecycle of the waste containers,
                 •   Derive container functions
                 •   Analyse and compile the possible loads, effects, and processes
                 •   Eventually create generic concepts

March 11, 2021                          WMSymposia2021|Wilhelm Bollingerfehr, et. al.   10
Methodological Approach

                                                                                                 ©2021 BGE TECHNOLOGY GmbH
 • Siting process in Germany = a stepwise approach
 • Derivation of container requirements as well
            First general, than host rock specific, eventually site specific

March 11, 2021                              WMSymposia2021|Wilhelm Bollingerfehr, et. al.   11
Fundamental Container Requirements
 Six fundamental requirements, all of them initially independent of the host rock:

                                                                                          ©2021 BGE TECHNOLOGY GmbH
       Confinement of the radioactive inventory,
       Shielding of ionising radiation,
       Exclusion of criticality,
       Temperature limitation of the waste container,
       Limitation of corrosion and gas production,
       Handleability

March 11, 2021                      WMSymposia2021|Wilhelm Bollingerfehr, et. al.    12
Phases of a Repository Life Time
       Phase 1:
        Emplacement phase (provision of the container for emplacement until emplacement of

                                                                                                        ©2021 BGE TECHNOLOGY GmbH
        the container is completed)
       Phase 2:
        Retrievability phase (completion of emplacement of the container until start of
        decommissioning of the repository)
       Phase 3:
        Recoverability phase (start of decommissioning of the repository until 500 years after
        closure of the repository)
       Phase 4:
        Later post-operational phase (500 years after closure of the repository until the end of
        the reference period)

March 11, 2021                          WMSymposia2021|Wilhelm Bollingerfehr, et. al.              13
Basic Container Requirements (e.g. for crystalline rock)
                                                                                       Time phase
       Basic Requirement
                                Emplacement                      Retrievability                          Recovery                      Later post-operation
                                                                                                To be sufficiently ensured for      Requirements depend on CRZ
       Containment of the

                                                                                                                                                                     ©2021 BGE TECHNOLOGY GmbH
                                               To be fully ensured                             developments that are probable       (Containment Providing Rock
      radioactive inventory                                                                          or can be expected                       Zone)

                                                                                               To be sufficiently ensured for
                                To be sufficiently ensured for repository operation           developments that are probable
      Shielding of ionising
                                                                                                    or can be expected
            radiation
                                                          To be sufficiently ensured to avoid radiologically- or radiolytically-induced damage to further barriers

     Exclusion of criticality                           To be fully ensured for the most reactive arrangement of the nuclear fuel

                                                                                               To be sufficiently ensured for
     Temperature limitation     To be sufficiently ensured for repository operation           developments that are probable
                                                                                                    or can be expected
     Limitation of corrosion                                                  To be sufficiently ensured to prevent unacceptable corrosion
       and gas production                                                       in case of contact with the hydro-chemical environment

                                                                                                To be sufficiently ensured for
          Handleability                     To be sufficiently ensured                         developments that are probable
                                                                                                     or can be expected

March 11, 2021                                         WMSymposia2021|Wilhelm Bollingerfehr, et. al.                                                            14
Basic Container Requirements (e.g. for crystalline rock)
                                                                                       Time phase
       Basic Requirement
                                Emplacement                      Retrievability                          Recovery                      Later post-operation
                                                                                                To be sufficiently ensured for      Requirements depend on CRZ
       Containment of the

                                                                                                                                                                     ©2021 BGE TECHNOLOGY GmbH
                                               To be fully ensured                             developments that are probable       (Containment Providing Rock
      radioactive inventory                                                                          or can be expected                       Zone)

                                                                                               To be sufficiently ensured for
                                To be sufficiently ensured for repository operation           developments that are probable
      Shielding of ionising
                                                                                                    or can be expected
            radiation
                                                          To be sufficiently ensured to avoid radiologically- or radiolytically-induced damage to further barriers

     Exclusion of criticality                           To be fully ensured for the most reactive arrangement of the nuclear fuel

                                                                                               To be sufficiently ensured for
     Temperature limitation     To be sufficiently ensured for repository operation           developments that are probable
                                                                                                    or can be expected
     Limitation of corrosion                                                  To be sufficiently ensured to prevent unacceptable corrosion
       and gas production                                                       in case of contact with the hydro-chemical environment

                                                                                                To be sufficiently ensured for
          Handleability                     To be sufficiently ensured                         developments that are probable
                                                                                                     or can be expected

March 11, 2021                                         WMSymposia2021|Wilhelm Bollingerfehr, et. al.                                                            15
Quantification of Function: e.g. Temperature Limitation
     Type of Temperature                                             Explanation                               Source

                                                                                                                                   ©2021 BGE TECHNOLOGY GmbH
                                                                                                              Type B(U)
                           Max. 85°C for handleability
    Surface Temperature                                                                                   shipped item ADR,
                           50°C on touchable surfaces
                                                                                                                2017

    Surface Temperature    100°C as preliminary surface temperature of waste container                     StandAG, 2017

                           200°C for Rock salt                                                                  VSG
    Surface Temperature
                           150°C for Claystone                                                               ANSICHT
                           100°C for Crystalline rock                                                     „KBS-3 Concept“

                                                                                                            Construction
                           390°C for PWR-SF
    Temperature of                                                                                       documents POLLUX®,
                           410°C for BWR-Sf
    Inventory                                                                                                   1986
                           500°C for glass of vitrified waste
                                                                                                             FZKA, 2001

March 11, 2021                                           WMSymposia2021|Wilhelm Bollingerfehr, et. al.                        16
Quantification of Function: e.g. Temperature Limitation
     Type of Temperature                                             Explanation                               Source

                                                                                                                                   ©2021 BGE TECHNOLOGY GmbH
                                                                                                              Type B(U)
                           Max. 85°C for handleability
    Surface Temperature                                                                                   shipped item ADR,
                           50°C on touchable surfaces
                                                                                                                2017

    Surface Temperature    100°C as preliminary surface temperature of waste container                     StandAG, 2017

                           200°C for Rock salt                                                                  VSG
    Surface Temperature
                           150°C for Claystone                                                               ANSICHT
                           100°C for Crystalline rock                                                     „KBS-3 Concept“

                                                                                                            Construction
                           390°C for PWR-SF
    Temperature of                                                                                       documents POLLUX®,
                           410°C for BWR-Sf
    Inventory                                                                                                   1986
                           500°C for glass of vitrified waste
                                                                                                             FZKA, 2001

March 11, 2021                                           WMSymposia2021|Wilhelm Bollingerfehr, et. al.                        17
Classification of Relevant Impacts on Waste Containers
                 Impact class             Nature of the relevant impact                                      Possible consequences
                                                                       Rock pressure,
                                                             Swelling pressure, Water pressure
                                                                   (isotropic, anisotropic)

                                                                                                                                                      ©2021 BGE TECHNOLOGY GmbH
                                 Static
                                                                           Shear
                                                                         Assembly;                         Material or component failure;
                 Mechanical                                              Handling
                                                                                                           Danger to the safety functions
                                                            Accelerations, vibrations, shocks from
                                                             handling and repository operation
                                Dynamic
                                                           Accident scenarios, e.g. container crash
                                           Decay heat of radioactive waste
                                                                                                           Thermal damage to technical,
                  Thermal                        Rock temperature
                                                                                                       geotechnical and/or geological barriers
                                                   Accident fire
                                                                                                      Material embrittlement / decomposition;
                 Radiological              Gamma and neutron radiation                                        Radiolysis gas formation

                                                                                                                     Corrosion
                                                  Corrosive media                                             Material decomposition
             Chemical and
                                                     Free water                                               Hydrogen embrittlement
              Biological
                                                  Microorganisms                                              Stress corrosion cracking
                                                                                                                   Gas formation

March 11, 2021                            WMSymposia2021|Wilhelm Bollingerfehr, et. al.                                                          18
Classification of Relevant Impacts on Waste Containers
                 Impact class             Nature of the relevant impact                                      Possible consequences
                                                                       Rock pressure,
                                                             Swelling pressure, Water pressure
                                                                   (isotropic, anisotropic)

                                                                                                                                                      ©2021 BGE TECHNOLOGY GmbH
                                 Static
                                                                           Shear
                                                                         Assembly;                         Material or component failure;
                 Mechanical                                              Handling
                                                                                                           Danger to the safety functions
                                                            Accelerations, vibrations, shocks from
                                                             handling and repository operation
                                Dynamic
                                                           Accident scenarios, e.g. container crash
                                           Decay heat of radioactive waste
                                                                                                           Thermal damage to technical,
                  Thermal                        Rock temperature
                                                                                                       geotechnical and/or geological barriers
                                                   Accident fire
                                                                                                      Material embrittlement / decomposition;
                 Radiological              Gamma and neutron radiation                                        Radiolysis gas formation

                                                                                                                     Corrosion
                                                  Corrosive media                                             Material decomposition
             Chemical and
                                                     Free water                                               Hydrogen embrittlement
              Biological
                                                  Microorganisms                                              Stress corrosion cracking
                                                                                                                   Gas formation

March 11, 2021                            WMSymposia2021|Wilhelm Bollingerfehr, et. al.                                                          19
Transferability of international Container Concepts

                                                                            ©2021 BGE TECHNOLOGY GmbH
March 11, 2021         WMSymposia2021|Wilhelm Bollingerfehr, et. al.   20
Transferability of international Container Concepts

                                                                                                   ©2021 BGE TECHNOLOGY GmbH
        In principle transfer of concepts possible – however, national requirements prevail

March 11, 2021                         WMSymposia2021|Wilhelm Bollingerfehr, et. al.          21
Solution Matrix for Container Concepts

                                                                           ©2021 BGE TECHNOLOGY GmbH
March 11, 2021        WMSymposia2021|Wilhelm Bollingerfehr, et. al.   22
Solution Matrix for Container Concepts

                                                                           ©2021 BGE TECHNOLOGY GmbH
March 11, 2021        WMSymposia2021|Wilhelm Bollingerfehr, et. al.   23
Schematic Diagram of Generic Container Concepts
                                                                                                                                          chosen technical solution for neutron shielding
                                                                                                                             without moderator material                 with moderator material
       Material of the
                                                                                                                             cast steel            cast iron          cast steel            cast iron
       inner container

                                                                                                                                                                                                                                                                                                            ©2021 BGE TECHNOLOGY GmbH
        Sketches of possible container concepts for final disposal in host rock...

                                                                                     crystalline rock

                                                                                                        Without
                                                                                                         CRZ
                                                                                                        CRZ
                                                                                                        with
                                                                                     stone
                                                                                     clay-

                                                                                                        corrosion
                                                                                                          with
                                                                                     rock salt

                                                                                                         without corrosion

                                                                                                                                                                                                                                                                           corrosion protection
                                                                                                                                                                                                                                                               stainless
                                                                                                                                                                                                               Colour legend   cast iron       (cast) Steel                (copper, titanium, nickel
                                                                                                                                                                                                                                                               steel
                                                                                                                                                                                                                                                                           alloy)

                                                                                                                                                                                                                               inventory   ●   moderator rod (exemplary)

March 11, 2021                                                                                                                                                                     WMSymposia2021|Wilhelm Bollingerfehr, et. al.                                                                       24
Conclusions & Recommendations
 1. Continuous monitoring of international waste container concept developments

 2. Improvement of geological database for potential repository sites

                                                                                              ©2021 BGE TECHNOLOGY GmbH
 3. Concretisation of the site-specific requirements for waste container

 4. Concretisation of the operation-related impacts on waste container

 5. Development of decision criteria for suitable repository concepts

 6. Preference: robust container concepts, proven and tested materials and technologies

 7. Start of development of container concepts for claystone and crystalline rock asap

March 11, 2021                    WMSymposia2021|Wilhelm Bollingerfehr, et. al.          25
Acknowledgement

 KoBrA-project:

                                                                                   ©2021 BGE TECHNOLOGY GmbH
  Funded by the Federal Ministry for Economic Affairs and Energy (BMWi),
  Represented by the Project Management Agency Karlsruhe,
    Karlsruhe Institute of Technology (KIT)

 Project results available:
  Synthesis report in German and English
  4 technical reports

March 11, 2021                WMSymposia2021|Wilhelm Bollingerfehr, et. al.   26
©2021 BGE TECHNOLOGY GmbH
                 Thank you for your attention!
March 11, 2021          WMSymposia2021|Wilhelm Bollingerfehr, et. al.   27
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