Requirements and Concepts for Waste Containers for Heat-Generating Radioactive Waste and Spent Fuel in Rock Salt, Claystone, and Crystalline Rock
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Requirements and Concepts for Waste Containers for Heat-Generating Radioactive Waste and Spent Fuel in ©2021 BGE TECHNOLOGY GmbH Rock Salt, Claystone, and Crystalline Rock Wilhelm Bollingerfehr, Ansgar Wunderlich (BGE TECHNOLOGY GmbH) Sabine Prignitz (BGE Bundesgesellschaft für Endlagerung mbH) Holger Völzke, Christian Herold, Dietmar Wolff (Bundesanstalt für Materialforschung und –prüfung) WMSymposia2021 | Wilhelm Bollingerfehr et. al.
Context German Site Selection Act (StandAG) as of summer 2017: Repository systems for 3 host rock formations to be considered ©2021 BGE TECHNOLOGY GmbH Rock salt, claystone and crystalline rock Type and total amount of expected heat generating waste: Waste from reprocessing: approx. 8000 coquilles Spent nuclear fuel: approx. 10,500 t of HM Waste container considered as a pivotal barrier of the entire repository system Question: How to correctly derive requirements for waste containers designed for HLW and SF? March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 1
Status of HLW-Waste Container Development ©2021 BGE TECHNOLOGY GmbH POLLUX® 10 POLLUX® 3 real existing waste container idea of a waste container without any (prototype), detailed planning manufactured on the basis of adjusted for a repository concept in detailed design calculations claystone March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 2
Status of HLW-Waste Container Development ©2021 BGE TECHNOLOGY GmbH POLLUX® 10 POLLUX® 3 real existing waste container idea of a waste container without any (prototype), detailed planning manufactured on the basis of adjusted for a repository concept in detailed design calculations claystone March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 3
R&D-Project KoBrA In summer 2017 BMWi launched the R&D-Project: „Requirements and concepts for waste containers for the disposal of heat generating radioactive waste and spent nuclear fuel in rock salt, claystone and crystalline rock“ ©2021 BGE TECHNOLOGY GmbH („Anforderungen und Konzepte für Behälter zur Endlagerung von Wärme entwickelnden radioaktiven Abfällen und ausgedienten Brennelementen in Steinsalz, Tonstein und Kristallingestein“ – Acronym: KoBrA) Project partners: BAM (Bundesanstalt für Materialforschung und –prüfung), Berlin and BGE TECHNOLOGY GmbH, Peine (coordinator) Project duration: July 2017 to April 2020 March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 4
Work Program 1. Survey of international existing requirements and concepts for waste container ©2021 BGE TECHNOLOGY GmbH 2. Identification of waste container-relevant boundary conditions and load parameter 3. Derivation and compilation of requirements for waste containers 4. Development of ideas and concepts for waste container designs March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 5
Waste Container Worldwide Host rock Container concept (Developers) Description Status of development well advanced in the licensing KBS-3 unshielded double-hull cask (cast-iron cask with solid procedure (tests for production, (SKB/Posiva Oy, Sweden, Finland) copper cladding) for fuel assemblies loading, sealing, transport, ©2021 BGE TECHNOLOGY GmbH storage) concept study derived from KBS- Crystalline Rock UOS unshielded double-hull cask made of different steels for fuel 3 (Škoda, Czech Rep.) assemblies ("KBS-3 made of steel") UFC II unshielded steel container with thin copper coating for advanced concept (material, (NWMO, Canada) (CANDU) fuel assemblies production and container tests) Category C Container advanced concept (material, unshielded steel canisters or fuel assemblies (Andra, France) production and container tests) Supercontainer steel cask for fuel assemblies or HLW canisters enclosed in Claystone Material tests (ONDRAF/NIRAS, Belgium) concrete generic design for fuel assemblies and canisters Reference container unshielded, robust steel container for fuel assemblies or considered by RWM as a (Nagra, Switzerland) HLW canisters possible reference concept for final disposal containers in salt BSK-3 Concept developed in R&D unshielded steel canisters for the borehole storage of drawn Rock salt reports; emplace-ment (GNS, Germany) fuel rods or HLW canisters technology tested on dummy POLLUX®-10 advanced concept (POLLUX®-8 shielded double-hull cask (steel and cast iron) for drawn fuel manufactured as prototype; (GNS, Germany) rods or HLW canisters storage technology tested) Existing containers; Transport and Storage Casks, e.g. CASTOR® shielded transport and interim storage casks made of cast -- suitability for final disposal not yet (GNS, Germany) iron or forged steel for fuel assemblies or HLW canisters considered March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 6
Waste Container Boundary Conditions 2. concepts for a repository in claystone ©2021 BGE TECHNOLOGY GmbH 1. concept for a repository in rocksalt German French Repository Concept Repository Concept (R&D-Project: AnSicht) (Source: Andra) Source: SKB 3. concept for a repository in crystalline rock March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 7
Waste Container Boundary Conditions 2. concepts for a repository in claystone ©2021 BGE TECHNOLOGY GmbH 1. concept for a repository in rocksalt But how to derive correctly a comprehensive set of requirements for waste containers for different host rocks? German French Repository Concept Repository Concept (R&D-Project: AnSicht) (Source: Andra) Source: SKB 3. concept for a repository in crystalline rock March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 8
Methodological Approach ©2021 BGE TECHNOLOGY GmbH March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 9
Methodological Approach ©2021 BGE TECHNOLOGY GmbH The idea is to: • Start with a compilation of requirements (regulatory, etc.) • Consider the lifecycle of the waste containers, • Derive container functions • Analyse and compile the possible loads, effects, and processes • Eventually create generic concepts March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 10
Methodological Approach ©2021 BGE TECHNOLOGY GmbH • Siting process in Germany = a stepwise approach • Derivation of container requirements as well First general, than host rock specific, eventually site specific March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 11
Fundamental Container Requirements Six fundamental requirements, all of them initially independent of the host rock: ©2021 BGE TECHNOLOGY GmbH Confinement of the radioactive inventory, Shielding of ionising radiation, Exclusion of criticality, Temperature limitation of the waste container, Limitation of corrosion and gas production, Handleability March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 12
Phases of a Repository Life Time Phase 1: Emplacement phase (provision of the container for emplacement until emplacement of ©2021 BGE TECHNOLOGY GmbH the container is completed) Phase 2: Retrievability phase (completion of emplacement of the container until start of decommissioning of the repository) Phase 3: Recoverability phase (start of decommissioning of the repository until 500 years after closure of the repository) Phase 4: Later post-operational phase (500 years after closure of the repository until the end of the reference period) March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 13
Basic Container Requirements (e.g. for crystalline rock) Time phase Basic Requirement Emplacement Retrievability Recovery Later post-operation To be sufficiently ensured for Requirements depend on CRZ Containment of the ©2021 BGE TECHNOLOGY GmbH To be fully ensured developments that are probable (Containment Providing Rock radioactive inventory or can be expected Zone) To be sufficiently ensured for To be sufficiently ensured for repository operation developments that are probable Shielding of ionising or can be expected radiation To be sufficiently ensured to avoid radiologically- or radiolytically-induced damage to further barriers Exclusion of criticality To be fully ensured for the most reactive arrangement of the nuclear fuel To be sufficiently ensured for Temperature limitation To be sufficiently ensured for repository operation developments that are probable or can be expected Limitation of corrosion To be sufficiently ensured to prevent unacceptable corrosion and gas production in case of contact with the hydro-chemical environment To be sufficiently ensured for Handleability To be sufficiently ensured developments that are probable or can be expected March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 14
Basic Container Requirements (e.g. for crystalline rock) Time phase Basic Requirement Emplacement Retrievability Recovery Later post-operation To be sufficiently ensured for Requirements depend on CRZ Containment of the ©2021 BGE TECHNOLOGY GmbH To be fully ensured developments that are probable (Containment Providing Rock radioactive inventory or can be expected Zone) To be sufficiently ensured for To be sufficiently ensured for repository operation developments that are probable Shielding of ionising or can be expected radiation To be sufficiently ensured to avoid radiologically- or radiolytically-induced damage to further barriers Exclusion of criticality To be fully ensured for the most reactive arrangement of the nuclear fuel To be sufficiently ensured for Temperature limitation To be sufficiently ensured for repository operation developments that are probable or can be expected Limitation of corrosion To be sufficiently ensured to prevent unacceptable corrosion and gas production in case of contact with the hydro-chemical environment To be sufficiently ensured for Handleability To be sufficiently ensured developments that are probable or can be expected March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 15
Quantification of Function: e.g. Temperature Limitation Type of Temperature Explanation Source ©2021 BGE TECHNOLOGY GmbH Type B(U) Max. 85°C for handleability Surface Temperature shipped item ADR, 50°C on touchable surfaces 2017 Surface Temperature 100°C as preliminary surface temperature of waste container StandAG, 2017 200°C for Rock salt VSG Surface Temperature 150°C for Claystone ANSICHT 100°C for Crystalline rock „KBS-3 Concept“ Construction 390°C for PWR-SF Temperature of documents POLLUX®, 410°C for BWR-Sf Inventory 1986 500°C for glass of vitrified waste FZKA, 2001 March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 16
Quantification of Function: e.g. Temperature Limitation Type of Temperature Explanation Source ©2021 BGE TECHNOLOGY GmbH Type B(U) Max. 85°C for handleability Surface Temperature shipped item ADR, 50°C on touchable surfaces 2017 Surface Temperature 100°C as preliminary surface temperature of waste container StandAG, 2017 200°C for Rock salt VSG Surface Temperature 150°C for Claystone ANSICHT 100°C for Crystalline rock „KBS-3 Concept“ Construction 390°C for PWR-SF Temperature of documents POLLUX®, 410°C for BWR-Sf Inventory 1986 500°C for glass of vitrified waste FZKA, 2001 March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 17
Classification of Relevant Impacts on Waste Containers Impact class Nature of the relevant impact Possible consequences Rock pressure, Swelling pressure, Water pressure (isotropic, anisotropic) ©2021 BGE TECHNOLOGY GmbH Static Shear Assembly; Material or component failure; Mechanical Handling Danger to the safety functions Accelerations, vibrations, shocks from handling and repository operation Dynamic Accident scenarios, e.g. container crash Decay heat of radioactive waste Thermal damage to technical, Thermal Rock temperature geotechnical and/or geological barriers Accident fire Material embrittlement / decomposition; Radiological Gamma and neutron radiation Radiolysis gas formation Corrosion Corrosive media Material decomposition Chemical and Free water Hydrogen embrittlement Biological Microorganisms Stress corrosion cracking Gas formation March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 18
Classification of Relevant Impacts on Waste Containers Impact class Nature of the relevant impact Possible consequences Rock pressure, Swelling pressure, Water pressure (isotropic, anisotropic) ©2021 BGE TECHNOLOGY GmbH Static Shear Assembly; Material or component failure; Mechanical Handling Danger to the safety functions Accelerations, vibrations, shocks from handling and repository operation Dynamic Accident scenarios, e.g. container crash Decay heat of radioactive waste Thermal damage to technical, Thermal Rock temperature geotechnical and/or geological barriers Accident fire Material embrittlement / decomposition; Radiological Gamma and neutron radiation Radiolysis gas formation Corrosion Corrosive media Material decomposition Chemical and Free water Hydrogen embrittlement Biological Microorganisms Stress corrosion cracking Gas formation March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 19
Transferability of international Container Concepts ©2021 BGE TECHNOLOGY GmbH March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 20
Transferability of international Container Concepts ©2021 BGE TECHNOLOGY GmbH In principle transfer of concepts possible – however, national requirements prevail March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 21
Solution Matrix for Container Concepts ©2021 BGE TECHNOLOGY GmbH March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 22
Solution Matrix for Container Concepts ©2021 BGE TECHNOLOGY GmbH March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 23
Schematic Diagram of Generic Container Concepts chosen technical solution for neutron shielding without moderator material with moderator material Material of the cast steel cast iron cast steel cast iron inner container ©2021 BGE TECHNOLOGY GmbH Sketches of possible container concepts for final disposal in host rock... crystalline rock Without CRZ CRZ with stone clay- corrosion with rock salt without corrosion corrosion protection stainless Colour legend cast iron (cast) Steel (copper, titanium, nickel steel alloy) inventory ● moderator rod (exemplary) March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 24
Conclusions & Recommendations 1. Continuous monitoring of international waste container concept developments 2. Improvement of geological database for potential repository sites ©2021 BGE TECHNOLOGY GmbH 3. Concretisation of the site-specific requirements for waste container 4. Concretisation of the operation-related impacts on waste container 5. Development of decision criteria for suitable repository concepts 6. Preference: robust container concepts, proven and tested materials and technologies 7. Start of development of container concepts for claystone and crystalline rock asap March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 25
Acknowledgement KoBrA-project: ©2021 BGE TECHNOLOGY GmbH Funded by the Federal Ministry for Economic Affairs and Energy (BMWi), Represented by the Project Management Agency Karlsruhe, Karlsruhe Institute of Technology (KIT) Project results available: Synthesis report in German and English 4 technical reports March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 26
©2021 BGE TECHNOLOGY GmbH Thank you for your attention! March 11, 2021 WMSymposia2021|Wilhelm Bollingerfehr, et. al. 27
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